Skip to main content

Thank you for visiting nature.com. You are using a browser version with limited support for CSS. To obtain the best experience, we recommend you use a more up to date browser (or turn off compatibility mode in Internet Explorer). In the meantime, to ensure continued support, we are displaying the site without styles and JavaScript.

  • NEWS AND VIEWS

A strange metal emerges from a failed superconductor

Above a certain temperature, the electrical resistance of copper–oxygen ceramic materials (called cuprates) increases in direct proportion to their temperature, reaching values far above the reasonable limits of electrical conduction1. This behaviour cannot be attributed to the way electrons usually interact with one another, or with atomic nuclei, and it has no widely accepted explanation — a trait that has given these materials the name of bad, or strange, metals. Writing in Nature, Yang et al.2 report this strange-metallic behaviour in a thin-film cuprate containing yttrium, barium, copper and oxygen (YBa2Cu3O7 − δ), in which nanopatterning enhances the disorder present in the material. Moreover, they find that this behaviour occurs at lower temperatures than expected, redrafting the accepted strange-metal blueprint.

The first surprises about cuprates emerged in 1986, when it was shown that they can be tuned to become magnetic or to carry electricity with zero resistance (superconduct) below a critical temperature that is much higher than physicists thought possible3. No unifying theory exists for these decades-old findings, but many researchers think that the materials’ strange-metallic behaviour presents an even greater puzzle.

Despite its inexplicability, strange-metallic behaviour seems to be everywhere. Enormous efforts are being made to derive a rigorous theory that explains why it shows up in a range of materials — from iron-based superconductors4 to ruthenium-based compounds5 and twisted bilayer graphene, in which each layer is a single sheet of carbon atoms and the layers are twisted relative to each other6. These solids all host exotic phenomena, such as high-temperature superconductivity, which makes the occurrence of strange-metallic behaviour in these systems all the more intriguing7. It is tempting to assume that something ties them all together.

So what makes a metal strange? Common electronic states of matter — ordinary metals, semiconductors and insulators — can all be described using electrons as the fundamental building block of the state. When electrons interact with one another in ordinary metals, they induce an electrical resistance that varies with the square of the temperature. But strange metals are different: as well as having an electrical resistance that scales proportionally with temperature, when these metals are subjected to a magnetic field, this resistance sometimes also increases linearly with the strength of the field8.

Yang et al. saw just this behaviour in thin films of YBa2Cu3O7 − δ, which would otherwise be superconducting below a critical temperature. The authors drilled a triangular array of nanometre-sized holes in the films using reactive-ion etching, a kind of atomic sandblasting (Fig. 1). The thinness of the film, combined with these holes, introduced disorder into the system, and this disorder is known to suppress the superconductivity9 — a trait for which such materials are sometimes known as failed superconductors. The lattice of holes left behind an array of connected island nodes, and Yang et al. showed that the electrical resistance exhibited linear dependence on both temperature and magnetic field strength. In doing so, the authors showed that this material can transition from a failed superconductor to a strange metal.

figure 1

Figure 1 | A strange metal exhibits oscillations in electrical resistance. Yang et al.2 drilled an array of nanometre-sized holes in thin films of the cuprate material YBa2Cu3O7 − δ grown on a substrate (strontium titanate), resulting in a pattern of connected islands. In a magnetic field, the quantum nature of the electrons on such islands makes it energetically favourable to have an integer number of magnetic-flux lines through each hole. When the field strength takes non-integer values, the cuprate’s electrical resistance increases, resulting in oscillations as the field strength is changed. Yang et al. measured such oscillations in the electrical resistance of YBa2Cu3O7 − δ and found that the oscillation amplitude increased with decreasing temperature. These oscillations have not been seen before in a material, such as YBa2Cu3O7 − δ, hosting strange-metallic behaviour, in which electrical resistance increases linearly with temperature. (Adapted from Fig. 1 in ref. 2.)

To understand why this finding stretches the collective imagination about strange metals, it’s helpful to know a little more about how electrons behave in solids. Electrons are fermions, named after Italian physicist Enrico Fermi, which are particles that are characterized by having a spin (associated with intrinsic angular momentum) that takes half-integer values. By contrast, particles known as bosons, after Indian physicist Satyendra Nath Bose, have integer spin. So far, strange-metallic behaviour has been observed only under conditions in which electrons were originally thought to behave individually (as fermions), or collectively, through a quantum-mechanical property known as entanglement10,11.

But theories of superconductivity rely on the idea that pairs of electrons can be described as composite particles that act like bosons with integer spin. And materials with superconducting (and hence bosonic) character show a peculiar response to applied magnetic fields when disorder is introduced with a microscopic pattern of holes12. The quantum nature of the bosons on the islands requires that an integer number of magnetic-flux lines threads through the holes — each carrying a quantum of magnetic flux (Fig. 1). When the applied magnetic field lies between these integer values, the material’s electrical resistance increases. The result is a bosonic calling card: oscillations of resistance with changing magnetic field strength. And Yang and co-workers’ sample showed precisely this response below the critical temperature for superconductivity — offering direct evidence that a strange metal exhibits electronic transport with bosonic character.

The leading theoretical descriptions of strange metals are as varied as the materials that show strange-metallic behaviour — some even draw on surprising connections to black-hole physics13,14 — but a consensus model has yet to emerge. Possible connections to an underlying anomalous metallic phase are even more speculative. As the temperature approaches zero, the electrical resistance of many disordered 2D superconductors reaches a constant, non-zero value — but this behaviour is impossible according to theories that describe non-interacting electrons. Sometimes termed a bose metal, this anomalous state is similarly in need of a consensus microscopic theory, despite more than two decades of theoretical and experimental attempts to devise one15. Conclusive evidence that an anomalous metal lies at the zero-temperature limit of a strange metal would be a major result.

The present study leaves several questions open. First, on a technical level, it seems that control of the patterning process was key to Yang and colleagues’ findings. An earlier paper by members of the same group reported a similar system16, but strange-metallic behaviour was observed in the present study only when the patterning was made more uniform than that of the previous study2. Quantitative investigation of the interactions between nodes could address this issue.

Second, assuming that strange-metallic behaviour can lurk in sufficiently disordered superconductors, why hasn’t it been routinely observed in the panoply of materials and systems studied so far? An experiment reported last year counters this concern: nanopatterned films of the superconductor iron selenide also show electrical resistance with a linear dependence on temperature, suggesting another instance of strange-metallic behaviour in a system characterized by bosons17.

These findings are as fascinating as they might be challenging to reconcile. The work of Yang et al. represents an intriguing opportunity to unite two frontiers — strange metals and disordered superconductors — whose collective description would represent a major step forward for condensed-matter physics.

Nature 601, 198-199 (2022)

doi: https://doi.org/10.1038/d41586-021-03831-6

References

  1. Gurvitch, M. & Fiory, A. T. Phys. Rev. Lett. 59, 1337–1340 (1987).

    PubMed  Article  Google Scholar 

  2. Yang, C. et al. Nature 601, 205–210 (2022).

    Article  Google Scholar 

  3. Bednorz, J. G. & Müller, K. A. Z. Phys. B 64, 189–193 (1986).

    Article  Google Scholar 

  4. Kasahara, S. et al. Phys. Rev. B 81, 184519 (2010).

    Article  Google Scholar 

  5. Bruin, J. A. N., Sakai, H., Perry, R. S. & Mackenzie, A. P. Science 339, 804–807 (2013).

    PubMed  Article  Google Scholar 

  6. Cao, Y. et al. Phys. Rev. Lett. 124, 076801 (2020).

    PubMed  Article  Google Scholar 

  7. Keimer, B., Kivelson, S. A., Norman, M. R., Uchida, S. & Zaanen, J. Nature 518, 179–186 (2015).

    PubMed  Article  Google Scholar 

  8. Hayes, I. M. et al. Nature Phys. 12, 916–919 (2016).

    Article  Google Scholar 

  9. Goldman, A. M. & Marković, N. Phys. Today 51, 39–44 (1998).

    Article  Google Scholar 

  10. Varma, C. M., Littlewood, P. B., Schmitt-Rink, S., Abrahams, E. & Ruckenstein, A. E. Phys. Rev. Lett. 63, 1996–1999 (1989).

    PubMed  Article  Google Scholar 

  11. Sachdev, S. & Ye, J. Phys. Rev. Lett. 70, 3339–3342 (1993).

    PubMed  Article  Google Scholar 

  12. Stewart, M. D. Jr, Yin, A., Xu, J. M. & Valles, J. M. Jr Science 318, 1273–1275 (2007).

    PubMed  Article  Google Scholar 

  13. McGreevy, J. Physics 3, 83 (2010).

    Article  Google Scholar 

  14. Hartnoll, S. A. Nature Phys. 11, 54–61 (2015).

    Article  Google Scholar 

  15. Kapitulnik, A., Kivelson, S. A. & Spivak, B. Rev. Mod. Phys. 91, 011002 (2019).

    Article  Google Scholar 

  16. Yang, C. et al. Science 366, 1505–1509 (2019).

    PubMed  Article  Google Scholar 

  17. Li, Y. et al. Preprint at https://arxiv.org/abs/2111.15488 (2021).

Download references

Competing Interests

The author declares no competing interests.

Subjects

Nature Careers

Jobs

Nature Briefing

Sign up for the Nature Briefing newsletter — what matters in science, free to your inbox daily.

Get the most important science stories of the day, free in your inbox. Sign up for Nature Briefing

Search

Quick links